anger Susan broke the dish on purpose to show her anger.
antagonize Layla tried to antagonize Sami a little bit.
enrage Don't do it, please. It could enrage Tom even more.
exasperate Sorry, I didn't mean to exasperate you with my endless questions.

Popularity over time

Use in printed books, per decade from 1850 to 2019.

By length

3 letters: mad¹, irk¹
4 letters: wild¹, gall¹, rile¹
5 letters: angry², anger², annoy², rouse¹, rabid²
6 letters: savage², fierce¹, offend², raging², madden², raving², fuming², enrage², rankle²
7 letters: furious³, outrage², provoke², incense², enraged², frantic², inflame², envenom
8 letters: irritate³, frenzied², embitter³
9 letters: ferocious³, aggravate³
10 letters: outrageous³, exacerbate⁴, antagonize⁴, antagonise, exasperate⁴

The small number after each word is its number of syllables (angry² = 2 syllables).